The best CR you can get with the bore and stroke given is 9.15:1 with a zero deck, flat top pistons, comp gasket, and the heads cut .011 for 67 cc chambers. Y's came with deck clearance of .015-.020. The Aftermarket cast pistons commonly used, added another .015-.020 to the deck clearance. So the point is, achieving that 9.15:1 ratio is a challenge. OEM steel headgaskets are .023 thick, a savings of .018+. Most people say they are a bad idea but I still dont know exactly why. Maybe the Y's have less head bolt clamping than the Chevys.If you are really getting into the CR stuff, make sure to have each chamber CCd and adjusted as far as possible to equal volumes.
Regarding increasing intake or exhaust valve size: It seems to me that if you look at some of the other popular motors and their displacements, the intake valve/displacement size of the Y is generous using the 1.92 valves. Therefore I would also look at the exhaust valves and system first.